Protein docking and modelling

 

Protein docking is a computational method that aims to predict the structure of a protein-protein complex starting from the crystallographic coordinates of the single components by performing an exhaustive search of all possible configurations of the two partners.

 

 

Azurin-cytocrome C551 complex

 

 

Computational methods have been used to model the interaction between Azurin, an electron transfer protein from the opportunistic bacterium Pseudomonas aeruginosa, and its partner cytC551; an experimental investigation being made difficult by the transient character of the complex.

 

(Bizzarri AR, Brunori E, Bonanni B, Cannistraro S. Docking and molecular dynamics simulation of the Azurin–Cytochrome c551 electron transfer complex. J. Mol. Recognit. 2007; 20: 122–131)

 

 

 

 

 

 

Azurin-p53 complex

 

In the last decade it has been found that the bacterial protein Azurin is able to penetrate cancerous cells and inhibits their uncontrolled proliferation. Surprisingly the Azurin anticancer activity is connected with its interaction with the well known tumour suppressor p53 which should be stabilized and reactivated in cancer cells just by azurin. In this context, we have used computational docking to model the interaction of Azurin with p53 domains, in order to elucidate the molecular details of the interaction connected with Azurin mode of action.

 

 

 

 

 

 

 

 

 

 

 

 

 

De Grandis V, Bizzarri AR, Cannistraro S. Docking study

and free energy simulation of the complex between

p53 DNA-binding domain and azurin. J. Mol. Recognit. 2007; 20: 215–226

 

 

 

 

 

 

 

 

 

 

 

 

Taranta M, Bizzarri AR, Cannistraro S. Modeling the interaction

between the N-terminal domain of the tumor suppressor

p53 and azurin. J. Mol. Recognit. 2009; 22: 215–222

 

 

Computational mutagenesis

 

Computational methods allow simulating the effects that point mutations could have on the structure and stability of a complex. By means of this procedure we have demonstrate the crucial role of two Azurin amino acidic residues for its interaction with p53. In such a way we have thus significantly contributed in the understanding of the Azurin/p53 complex structure and properties.

 

From Azurin to p28

 

 

 

 

 

 

 

 

 

 

 

 

 

 

 

 

 

 

 

Three dimensional structure of Azurin. The cyan sequence corresponds to p28.

 

 

In the last two years the equip of scientist of the Division of Surgical Oncology of the University of Illinois College of Medicine of Chicago has found that the peptide fragment of azurin called p28, (residues 50 - 77 of the whole protein), retains both the cellular penetration ability and antiproliferative action of the whole protein (Yamada et al., 2009). As for azurin, the p28 antiproliferative activity is consequent to its interaction with p53.

Even if p28 has already entered the phase II clinical trials under the FDA allowance its mode of action has not been clarified mostly because the details of its interaction with p53 are unknown.

By means of computational docking procedure we have defined the molecular details of the interaction of p28 with the p53 core domain

 

 

 

 

 

 
thus contributing to open new perspectives on the possible p28 mode of action.

 

 

 
 

 

Three dimensional structure of the best p28-p23 core domain complex resulting from docking and molecular dynamics simulation procedures. (Santini S, Bizzarri AR, Cannistraro S. Modelling the interaction between the p53 DNA-binding domain and the p28 peptide fragment of Azurin. J. Mol. Recognit. 2011)